The automorphism group of an icosahedron -- the orientations of an icosahedron -- suggests a 60-card deck, or 120 if including reflections. 5 suits; 12 cards per suit. Each card could be annotated with its neighbors, and its antipode.
Unsure how to depict the group operation: two cards can be added to yield a third card. Maybe instead highlight the permutations of the alternating group A5.
Relatedly, the K6T deck has 120 cards; 20 in 6 suits.
The permutations of a 60 card deck can encode 272 bits; a 120-card deck 660 bits. 100 cards = 524 bits.
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